Nice!
I'm wondering if you aren't freezing the cooling liquid in the CPU cooler's heatpipes, leading to high temps!??
Sounds crazy right!

Bear with me:
Heatpipes work be boiling off liquid at the heat source (CPU)
The steam then flows to the cold side due to the suction caused by its condensing there, then the liquid flows back to the heat source by capillary action.
But
If the cold side is too cold; all the liquid will freeze there and capillary action will stop.
On the hot side there simply wont be any liquid to boil off.
That would explain your observations pretty well wouldn't it..?
Maybe a stock loop (Glycol excepted) is the better option...
The water volume will add to your 'Cold Battery'...
I'd add and extra pump or 2, in series, to keep the sludge moving/ impinging on the WB base.
Perhaps water in direct contact with end part of the evap is a better option than a stock rad..?
"end part":
You want to keep the air @ a lower temp than the water, just in case of condensation on the WB...
Oh ye;
I think moving the air is more important than you realize:
You want to reduce boundary layer thickness (aerodynamics), hence the fans on CPU coolers, rather than just relying on case airflow...
(That reminds me; Try a bigger fan on the DRAM and increase TREF a lot!)
The HVAC rule of thumb is to never have a fan closer to a perpendicular to airflow surface than the fan's diameter.
That means your evap rad is a bit too close to 'the wall' for optimal airflow through it.
Lets say said air is only in contact with the evap rad for half the time, but it'll be 'in contact' twice as often...