You should probably leave them how they are for now. But as you increase your FSB you will either have to increase your ram voltage, or slacken the timings a bit. your ram will eventually hit a wall where those timings will be too tight to run at a high FSB
i had a pair of DDR500 sticks that had timings of 3-4-4-8 and i tried to run them at 3-3-3-8 and i could only get an extra +20 to the FSB before windows would crash. i put it back down to 3-4-4-8 and ive gone as has as +80 on the FSB with a 1:1 on the mem
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